Abstract:

Aerosol-cloud interactions are a persistent source of uncertainty in climate research. This study presents findings from a model intercomparison project examining the impact of aerosols on clouds and climate in convection permitting Radiative-Convective Equilibrium (RCE) simulations. Specifically, 11 different modeling teams conducted RCE simulations under varying aerosol concentrations, domain configurations, and sea surface temperatures (SSTs). We analyze the response of domain-mean cloud and radiative properties to imposed aerosol concentrations across different SSTs. Additionally, we explore the potential impact of aerosols on convective aggregation and large-scale circulation in large-domain simulations.

The results reveal that the cloud and radiative responses to aerosols vary substantially across models. However, a common trend across models, SSTs, and domain configurations is that increased aerosol loading tends to suppress warm rain formation, enhance cloud water content in the mid-troposphere, and consequently increase mid-tropospheric humidity and upper-tropospheric temperature, thereby impacting static stability. The warming of the upper troposphere can be attributed to reduced lateral entrainment effects due to the higher environmental humidity in the mid-troposphere. However, models do not agree on aerosol impacts on convective updraft velocity based on the preliminary examination of high-percentiles of vertical velocity at a single mid-troposheric layer (500hPa). In large-domain simulations, where convection tends to self-organize, aerosol loading does not consistently influence self-organization but tends to reduce the intensity of large-scale circulation forming between convective clusters and dry regions. This reduction in circulation intensity can be explained by the increase in static stability due to the upper tropospheric warming.